Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20

ABSTRACT: FeGa3 is an unusual intermetallic semiconductor that presents intriguing magnetic responses to the tuning of its electronic properties. When doped with Ge, the system evolves from diamagnetic to paramagnetic to ferromagnetic ground states that are not well understood. In this work, we have...

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Autores:
Cabrera Baez, Michael
Naranjo Uribe, Andrés
Osorio Guillén, Jorge Mario
Rettori, Carlos
Ávila, Marco A.
Tipo de recurso:
Article of investigation
Fecha de publicación:
2015
Institución:
Universidad de Antioquia
Repositorio:
Repositorio UdeA
Idioma:
eng
OAI Identifier:
oai:bibliotecadigital.udea.edu.co:10495/7983
Acceso en línea:
http://hdl.handle.net/10495/7983
Palabra clave:
Electrónica
Electronics
Semiconductores
Semiconductors
Multibanda
Propiedades electrónicas
Rights
openAccess
License
https://creativecommons.org/licenses/by-nc-nd/4.0/
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network_acronym_str UDEA2
network_name_str Repositorio UdeA
repository_id_str
dc.title.spa.fl_str_mv Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20
title Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20
spellingShingle Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20
Electrónica
Electronics
Semiconductores
Semiconductors
Multibanda
Propiedades electrónicas
title_short Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20
title_full Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20
title_fullStr Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20
title_full_unstemmed Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20
title_sort Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20
dc.creator.fl_str_mv Cabrera Baez, Michael
Naranjo Uribe, Andrés
Osorio Guillén, Jorge Mario
Rettori, Carlos
Ávila, Marco A.
dc.contributor.author.none.fl_str_mv Cabrera Baez, Michael
Naranjo Uribe, Andrés
Osorio Guillén, Jorge Mario
Rettori, Carlos
Ávila, Marco A.
dc.contributor.researchgroup.spa.fl_str_mv Ciencia de los Materiales
dc.subject.lemb.none.fl_str_mv Electrónica
Electronics
Semiconductores
Semiconductors
topic Electrónica
Electronics
Semiconductores
Semiconductors
Multibanda
Propiedades electrónicas
dc.subject.proposal.spa.fl_str_mv Multibanda
Propiedades electrónicas
description ABSTRACT: FeGa3 is an unusual intermetallic semiconductor that presents intriguing magnetic responses to the tuning of its electronic properties. When doped with Ge, the system evolves from diamagnetic to paramagnetic to ferromagnetic ground states that are not well understood. In this work, we have performed a joint theoretical and experimental study of FeGa3−xGex using density functional theory and magnetic susceptibility measurements. For low Ge concentrations we observe the formation of localized moments on some Fe atoms and, as the dopant concentration increases, a more delocalized magnetic behavior emerges. The magnetic configuration strongly depends on the dopant distribution, leading even to the appearance of antiferromagnetic interactions in certain configurations.
publishDate 2015
dc.date.issued.none.fl_str_mv 2015
dc.date.accessioned.none.fl_str_mv 2017-08-18T16:39:36Z
dc.date.available.none.fl_str_mv 2017-08-18T16:39:36Z
dc.type.spa.fl_str_mv Artículo de investigación
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dc.identifier.citation.spa.fl_str_mv Cabrera Baez, M., Naranjo Uribe, A., Osorio Guillén, J. M., Rettori, C., & Ávila, M. A. (2015). Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20. Physical Review B: Condensed Matter. 92(214414), 1-9. DOI:10.1103/PhysRevB.92.214414
dc.identifier.issn.none.fl_str_mv 2469-9969
dc.identifier.uri.none.fl_str_mv http://hdl.handle.net/10495/7983
dc.identifier.doi.none.fl_str_mv 10.1103/PhysRevB.92.214414
dc.identifier.eissn.none.fl_str_mv 2469-9950
identifier_str_mv Cabrera Baez, M., Naranjo Uribe, A., Osorio Guillén, J. M., Rettori, C., & Ávila, M. A. (2015). Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20. Physical Review B: Condensed Matter. 92(214414), 1-9. DOI:10.1103/PhysRevB.92.214414
2469-9969
10.1103/PhysRevB.92.214414
2469-9950
url http://hdl.handle.net/10495/7983
dc.language.iso.spa.fl_str_mv eng
language eng
dc.relation.citationendpage.spa.fl_str_mv 9
dc.relation.citationissue.spa.fl_str_mv 214414
dc.relation.citationstartpage.spa.fl_str_mv 1
dc.relation.citationvolume.spa.fl_str_mv 92
dc.relation.ispartofjournal.spa.fl_str_mv Physical Review B: Condensed Matter
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dc.publisher.spa.fl_str_mv The American Physical Society
dc.publisher.place.spa.fl_str_mv Estados Unidos
institution Universidad de Antioquia
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spelling Cabrera Baez, MichaelNaranjo Uribe, AndrésOsorio Guillén, Jorge MarioRettori, CarlosÁvila, Marco A.Ciencia de los Materiales2017-08-18T16:39:36Z2017-08-18T16:39:36Z2015Cabrera Baez, M., Naranjo Uribe, A., Osorio Guillén, J. M., Rettori, C., & Ávila, M. A. (2015). Multiband electronic characterization of the complex intermetallic cage system Y1−xGdxCo2Zn20. Physical Review B: Condensed Matter. 92(214414), 1-9. DOI:10.1103/PhysRevB.92.2144142469-9969http://hdl.handle.net/10495/798310.1103/PhysRevB.92.2144142469-9950ABSTRACT: FeGa3 is an unusual intermetallic semiconductor that presents intriguing magnetic responses to the tuning of its electronic properties. When doped with Ge, the system evolves from diamagnetic to paramagnetic to ferromagnetic ground states that are not well understood. In this work, we have performed a joint theoretical and experimental study of FeGa3−xGex using density functional theory and magnetic susceptibility measurements. For low Ge concentrations we observe the formation of localized moments on some Fe atoms and, as the dopant concentration increases, a more delocalized magnetic behavior emerges. 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